The core of the archive constitutes the material that remained with E.H. Shepard following his donation of drawings and sketches to the Victoria and Albert Museum and the British Cartoon Archive: personal, business, and fan correspondence; personal and family papers; personal ephemera; copies of books he wrote or illustrated; appointment diaries; sketchbooks; photographs; pencil, ink, and watercolour drawings; oil paintings; manuscript material; press cuttings, sales catalogues, and magazines.
In addition, material accumulated by the University of Surrey relating to E.H. Shepard has been catalogued as part of this collection. This accumulated material includes later editions of works illustrated or written by Shepard; books and reference material about Shepard; some photographs of locations specific to Shepard's life; and artwork by Shepard donated by third parties.